Development of uranium reference particles to support nuclear safeguards

نویسندگان

  • E. A. Stefaniak
  • R. Kips
  • J. Truyens
  • Y. Aregbe
  • M. Kraiem
  • S. Richter
  • R. Wellum
چکیده

Controlled hydrolysis of certified uranium hexafluoride, carried out in a specifically constructed aerosol chamber, leads to the production of uranyl fluoride particulates which – deposited on a graphite planchet support may be used as a quality control reference material. The particle size and surface distribution depends on several parameters, such as the relative humidity inside the aerosol chamber and the concentration of gaseous uranium hexafluoride, determined by the distillation conditions. The best quality samples were obtained at RH ranging from 55 to 70% and low gas amount. These improvements for a single deposition were used to prepare a reference sample with two different uranium enrichments. Preliminary SIMS measurements proved good results with respect to both types of particles. It was also revealed that – in some cases – the micrometer size uranium particles are accompanied by a large uranium background.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

NUSIMEP-7: uranium isotope amount ratios in uranium particles.

The Institute for Reference Materials and Measurements (IRMM) has extensive experience in the development of isotopic reference materials and the organization of interlaboratory comparisons (ILC) for nuclear measurements in compliance with the respective international guidelines (ISO Guide 34:2009 and ISO/IEC 17043:2010). The IRMM Nuclear Signatures Interlaboratory Measurement Evaluation Progra...

متن کامل

Identification of uranium signatures relevant for nuclear safeguards and forensics

The paper describes the applicability of different characteristics (signatures) in nuclear safeguards and forensics for assessment of uranium material provenance in terms of production process. The study follows a uranium ore concentrate production from an ore to a U3O8 product. It turned out that rare-earth elemental pattern, radiochronometry (age of ore body and material production date), sul...

متن کامل

IRMM-1000a and IRMM-1000b uranium reference materials certified for the production date. Part I: methodology, preparation and target characteristics

The paper describes the preparation and production of the reference materials, IRMM-1000a and IRMM-1000b, certified for the production date based on the 230Th/234U radiochronometer in compliance with ISO Guide 34:2009. The production date of the reference materials corresponds to the last separation of 230Th from 234U, i.e. when the initial daughter nuclide content in the material was finally r...

متن کامل

Nuclear Archaeology for Gaseous Diffusion Enrichment Plants

The field of nuclear archaeology aims to develop the methods and tools to verify past production of fissile materials for military purposes, which may become necessary to support the verification of future arms control agreements that envision deeper cuts in the nuclear arsenals. Techniques have been successfully demonstrated for reconstructing historic plutonium production, especially in graph...

متن کامل

Management 48 th Annual Meeting of the Institute of Nuclear Materials Management

196 SAGSI: Its Role and Contribution to Safeguards Development ............................ 1 J. Carlson Abstract #163 Nuclear Issue of North Korea and Applicability of the IAEA Safeguards System to North Korea .................................................................................................. 6 K. Choe163 Nuclear Issue of North Korea and Applicability of the IAEA Safeguards Syst...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2010